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Ziel dieser Arbeit war es ein formalkinetisches Reaktionsmodell für den MTO-Prozess an AlPO4-gebundenen ZSM-5-Extrudaten zu erstellen. Dazu wurde eine Prozessstudie unter typischen MTO-Prozessbedingungen durchgeführt sowie ausgewählte Olefine einzeln und zusammen mit Methanol zudosiert. Anhand der experimentellen Daten konnte ein geeignetes Reaktionsnetz abgeleitet und ein Modell der Reaktionskinetik entwickelt werden.

Reaktionskinetik --- MTO-Prozess --- AlPO4-Binder --- Prozessstudie --- ZSM-5-Extrudate

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Microporous zeolites and nanoporous materials are important from an academic and industrial research perspective. These inorganic materials have found application as catalysts in several industrial processes in oil refinery, petro-chemical reactions, fine chemicals, speciality, drug discovery and pharmaceutical synthesis, exhaust emission control for stationary and mobile engines and industrial wastewater treatment. The reasons for their versatile applications in several industrial processes are their unique properties of microporous zeolites and nanoporous materials such as uniform pores, channel systems, shape selectivity, resistance to coke formation, thermal and hydrothermal stability. Furthermore, the possibility to tune the amount and strength of Brønsted and Lewis acid sites and their crystal size, as well as the possibility of modification with transition and noble metals, are key to their success as efficient, high selectivity and stable catalysts.

Technology: general issues --- Chemical engineering --- zeolitic imidazolate frameworks --- Zn-Co@N-doped carbon --- transesterification --- Ti-CFI --- Ti-CIT-5 --- extra-large-pore --- zeolites --- fluorides --- titanosilicates --- oxidation --- generalized macro-transport theory --- adsorbent and non-adsorbent membranes --- bulk and surface diffusion --- heterogeneous catalysis --- mass transfer and effectiveness factor --- mesoporous H-ZSM-5 --- methanol-to-olefin (MTO) --- propylene --- acid sites density --- operando UV-vis spectroscopy --- CO2 assisted dehydrogenation --- isobutane --- silicalite-1 --- SBA-15 --- carbamazepine --- ozone --- catalysts synthesis and characterization --- catalytic ozonation --- isosorbide --- solid acid catalyst --- sorbitol --- dehydration --- bisphenol A --- diclofenac --- heterogeneous catalyst --- catalyst characterization --- advanced oxidation processes --- methanol to aromatics --- para-xylene --- selectivity --- phosphorous modified ZSM-5 --- advanced oxidation process --- catalyst preparation --- wastewater treatment --- interzeolite conversion method --- CHA-type zeolite --- LTL-type zeolite --- crystallization mechanism --- MTO reaction --- α-Pinene oxide --- campholenic aldehyde --- trans-carveol --- isomerization --- MoO3-zeolite BETA --- n/a

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Microporous zeolites and nanoporous materials are important from an academic and industrial research perspective. These inorganic materials have found application as catalysts in several industrial processes in oil refinery, petro-chemical reactions, fine chemicals, speciality, drug discovery and pharmaceutical synthesis, exhaust emission control for stationary and mobile engines and industrial wastewater treatment. The reasons for their versatile applications in several industrial processes are their unique properties of microporous zeolites and nanoporous materials such as uniform pores, channel systems, shape selectivity, resistance to coke formation, thermal and hydrothermal stability. Furthermore, the possibility to tune the amount and strength of Brønsted and Lewis acid sites and their crystal size, as well as the possibility of modification with transition and noble metals, are key to their success as efficient, high selectivity and stable catalysts.

Technology: general issues --- Chemical engineering --- zeolitic imidazolate frameworks --- Zn-Co@N-doped carbon --- transesterification --- Ti-CFI --- Ti-CIT-5 --- extra-large-pore --- zeolites --- fluorides --- titanosilicates --- oxidation --- generalized macro-transport theory --- adsorbent and non-adsorbent membranes --- bulk and surface diffusion --- heterogeneous catalysis --- mass transfer and effectiveness factor --- mesoporous H-ZSM-5 --- methanol-to-olefin (MTO) --- propylene --- acid sites density --- operando UV-vis spectroscopy --- CO2 assisted dehydrogenation --- isobutane --- silicalite-1 --- SBA-15 --- carbamazepine --- ozone --- catalysts synthesis and characterization --- catalytic ozonation --- isosorbide --- solid acid catalyst --- sorbitol --- dehydration --- bisphenol A --- diclofenac --- heterogeneous catalyst --- catalyst characterization --- advanced oxidation processes --- methanol to aromatics --- para-xylene --- selectivity --- phosphorous modified ZSM-5 --- advanced oxidation process --- catalyst preparation --- wastewater treatment --- interzeolite conversion method --- CHA-type zeolite --- LTL-type zeolite --- crystallization mechanism --- MTO reaction --- α-Pinene oxide --- campholenic aldehyde --- trans-carveol --- isomerization --- MoO3-zeolite BETA

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Street Art Today is een actueel en eigentijds overzicht van de meest invloedrijke street artists, hun werk en de belangrijkste stromingen. De auteurs stelden deze who's who van de hedendaagse street art op in samenwerking met tal van kunstenaars. Namen als MOBSTR, Pixel Pancho, JR, 1010, Invader, spY passeren de revue.Exclusieve interviews, verhelderende essays en een voorwoord van Martyn Reed maken van dit boek een mustread voor al wie deze steeds populairder wordende kunstscene van ver of dichtbij volgt.

public spaces --- Contemporary [style of art] --- street art --- Art --- anno 2000-2009 --- anno 2010-2019 --- humor --- sculpture [visual works] --- mural paintings [visual works] --- site-specific works --- Walker, David --- Harrington, Conor --- Pixel Pancho --- M-City --- Levalet --- Nychos --- Void, Axel --- Inti --- Zacharevic, Ernest --- Hayuk, Maya --- Tenten/1010 --- Jana & Js --- Space Invader --- Iacurci, Agostino --- Os Gemeos --- Biancoshock --- Eversiempre --- Bicicleta Sem Freio --- Phlegm --- JR --- SpY --- Borondo --- Magee, Fintan --- DALeast --- Ella & Pitr --- Mobstr --- Strøk --- Fikos --- Faith 47 --- Escif --- Diaz, Alexis --- Aryz --- Cordal, Isaac --- MTO --- Etam Crew --- Bordalo II --- Ludo --- Helten, Van, Guido --- Elle --- Eaton, Tristan --- Case --- Telmo Miel --- Pejac --- ROA --- Rone --- Banksy --- Seth --- Iurato, Joe --- Hyuro --- Street art --- Art [Modern ] --- 21st century --- Mural painting and decoration --- Graffiti --- Muurschilderingen --- Beeldende kunst --- straatkunst --- urban art --- surrealisme --- toyisme --- naïeve kunst --- figuratieve kunst --- hyperrealisme --- urban interventionisme --- 738.9 --- schilder- en tekenkunst, overige genres en motieven -trompe l'oeil, graffiti --- Invader --- Muurschildering --- 730 --- grafische kunst --- art urbain --- schilder- en tekenkunst --- peinture et dessin --- kunst in de openbare ruimte --- social criticism --- Propaganda