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Zeolite membranes have shown promising applications in catalytic and separation processes in chemical industry. A simulation-assisted design method based on experiments and simulations is shown to guide the development of hierarchically structured catalyst systems based on zeolite membranes by predicting the optimal catalyst structure. A cornerstone of this method is a 3-D pore network model – crystallite-pore network model for simulation of diffusion and reaction in polycrystalline zeolites.

Direkte DME-Synthese --- Hochfrequenzschwingmikrowaage --- Kristallit-Porennetzwerk-Modell --- Crystallite-pore network model (CPNM) --- Direct DME-synthesis --- Polykristallines ZeolithCore-shell catalyst --- Polycrystalline zeolite --- High frequency oscillating microbalance --- Kern-Schale-Katalysator