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The properties and nature of water clusters studied with novel spectroscopic approaches are presented in this thesis. Following a general introduction on the chemistry of water and water clusters, detailed descriptions of the experiments and analyses are given. All the experimental results, including first size-selective spectra of large clusters consisting of 200 water molecules, are presented with corresponding analyses. Hitherto unidentified hydrogen bond network structures, dynamics, and reactivity of various water clusters have been characterized at the molecular level. The main targets of this book are physical chemists and chemical physicists who are interested in water chemistry or cluster chemistry.

Inorganic compounds. --- Hydrogen bonding --- Water --- Chemistry --- Physical Sciences & Mathematics --- Physical & Theoretical Chemistry --- Spectra --- Hydrogen bonding. --- Spectra. --- Hydrogen bonds --- Chemistry. --- Spectroscopy. --- Physical chemistry. --- Microscopy. --- Physical Chemistry. --- Spectroscopy and Microscopy. --- Spectroscopy/Spectrometry. --- Hydrology --- Chemistry, Physical and theoretical --- Molecular association --- Chemistry, Physical organic. --- Analysis, Spectrum --- Spectrochemical analysis --- Spectrochemistry --- Spectroscopy --- Chemistry, Analytic --- Interferometry --- Optics --- Radiation --- Wave-motion, Theory of --- Absorption spectra --- Light --- Spectroscope --- Chemistry, Physical organic --- Chemistry, Organic --- Qualitative --- Spectrometry --- Analysis, Microscopic --- Light microscopy --- Micrographic analysis --- Microscope and microscopy --- Microscopic analysis --- Optical microscopy --- Chemistry, Theoretical --- Physical chemistry --- Theoretical chemistry --- Analytical chemistry --- Water clusters --- Clusters, Water --- Molecules