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Laser powder bed fusion (LPBF) is one of the most common additive manufacturing (AM) techniques for fabricating various components in different industries. In recent years, fabricating a single component with a multi-material structure has become increasingly prevalent. It allows a combination of dissimilar materials with different properties into one component to obtain a unique function. However, the fabrication of multi-material parts with complex geometries via conventional methods is difficult due to their inherent limitations. Multi-material LPBF offers a new route for producing 3D objects with tailored properties. Despite its numerous advantages, the achievement of a free-defect interface between dissimilar materials can be the main challenge. Among multi-metallic materials, the stainless steel (SS)-copper (Cu) combination is very attractive due to the excellent thermal conductivity of Cu combined with the good mechanical properties and corrosion resistance of SS. This study explores the multi-material LPBF of 316L-CuCrZr components. The LPBF fabrication of SS-Cu multi-material parts is very challenging because of their significant difference in properties such as solubility, laser absorptivity, melting points, and thermal expansion coefficient, resulting in defects such as cracks and pores at the interface after LPBF processing. In this work, two potential techniques for resolving the interfacial defect issues were investigated. The first potential solution was surface modification of CuCrZr powder by chromium diffusion in a nitrogen atmosphere to increase the laser absorptivity of the copper-rich powder. The 316L-modified CuCrZr samples were printed in various conditions. Some SS-Cu samples were stacked horizontally with different scanning sequences and with different Cu printing parameters. In addition, some SS-Cu samples were stacked vertically with different CuCrZr LPBF scanning parameters, different interface designs and strategies, as well as the application of interface remelting strategies. In all samples, however, microcracks were observed at the interface between SS and Cu near the SS side, originating from Fe-rich regions. Another novel method to resolve the cracking problem was introducing a Ni-based interlayer. In this thesis, an Inconel 625 interlayer with variable thickness was deposited between the 316L and CuCrZr alloys. The microstructure, elemental distribution, and grain size and orientation of the multi-metallic samples were characterized. The results exhibited that the addition of a 40 µm thick interlayer does not have a tangible effect on eliminating crack formation. When increasing the interlayer thickness to 80 and 160 µm the number and size of microcracks significantly decreased in the Cu-Ni-Fe intermixing zone. The microcracks were mainly located at high-angle grain boundaries (>15°) and partially filled with copper. Finally, applying a Ni-based interlayer with a thickness of 240 µm could successfully eliminate the formation of microcracks. A further increase of the interlayer thickness to 320, 400, and 480 µm, still guaranteed the formation of crack-free interfaces. In all samples with Ni-based interlayers of at least 240 µm, no Fe was found near the interface between the Ni and Cu alloys, indicating that the interlayer thickness in crack-free samples was sufficient to avoid the presence of Fe-rich regions near the interface.
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