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Since the first works introducing the aluminum intercalated clay family in the early 1970s, interest in the synthesis of Pillared InterLayered Clays (PILC) has increased tremendously, especially research into their properties and energetic and environmental applications. After our comprehensive reviews and book on the synthesis and catalytic applications of these materials, new references have appeared in the literature and the interest in this field is continuously increasing. The aim of this Special Issue is to collect the recent advances developed considering this family of solids.

clays --- Al-PILC --- pillared clays --- scale up --- pillaring solution --- Keggin ion --- reutilization --- Keggin polycation --- concentrated media --- microwave radiation --- pillared montmorillonite --- AlNi-PILC --- Pd-Ce --- catalytic combustion --- benzene --- TPD/TPSR --- ZnO-TiO2/delaminated montmorillonite --- heterostructures --- Ag-coating --- solar photocatalytic activity --- water purification --- cadmium --- chitosan --- modification --- 13X molecular sieve --- removal --- dye remediation --- adsorption --- azo dye --- wastewater --- pillared porous phosphate heterostructures --- isotherm --- sericite --- thermal modification --- acid activation --- sodium modification --- montmorillonite/hydrotalcite composite --- montmorillonite/titania composite --- organoclay --- inverse micelle --- Mn-Al mixed oxide --- combustion catalysts --- ciprofloxacin --- smectite --- pillared clay --- keggin-like mixed Al/Fe polyoxocation --- mineralogical composition --- catalytic wet peroxide oxidation --- mesosilica --- methyl orange --- palygorskite